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Pure Appl. Chem., 2006, Vol. 78, No. 7, pp. 1341-1347

http://dx.doi.org/10.1351/pac200678071341

Syntheses and chemistry of bis- and tris-mercaptoborates

Sheldon G. Shore1, Ewan J. M. Hamilton2, Roman G. Kultyshev1, Hoitung T. Leung1 and Teshome Yisgedu1

1 Department of Chemistry, Ohio State University, Columbus, OH 43210, USA
2 Department of Chemistry, Ohio State University at Lima, Lima, OH 45804, USA

Abstract: The preparation and chemistry of bis- and tris-mercaptoborates based on closo-B12 and closo-B10 structures is described. These species undergo a number of reactions such as halogenation and alkylation without changing the closo-borane core. Addition of the third dimethylsulfide substituent to the closo-boranes is thought to proceed via an unusual cationic intermediate.